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4. "Love Me Harder" Featuring the Weeknd

Grande was a huge factor in the Weeknd's crossover from drugged-out alt-R&B king to a pop prince. His feature on the sultry, flirty duet "Love Me Harder" not only exposed him to a younger audience but was his first successful foray into Top 40 pop, which he would master with one of the Grande collab's co-writers Max Martin on "Can't Feel My Face" just months later.