'You Only Live Twice' (1967)
From the Eastern flavor of the opening theme, hauntingly sung by Nancy Sinatra, to the Japanese setting, the fifth film is the Bond series just gets better and cooler with age. The tasty script by Roald Dahl junks most of the Fleming novel, spinning its own witty Cold War fantasy. Connery's Bond finally gets to confront SPECTRE's arch-villain, Ernst Stavro Blofeld, previously unseen but now played to the creepy hilt by Donald Pleasance. Blofeld petting his white pussy while dropping enemies into a piranha pool spawned a trilogy of Austin Powers spoofs. And the chopper with a magnet to pick up assassins is a marvel.